A Novel Technology for Natural Gas Conversion by Means of Integrated Oxidative Coupling and Dry Reforming of Methane
Review
| Общее |
Language:
Английский,
Genre:
Review,
Status:
Published,
Source type:
Original
|
| Journal |
Chemie-Ingenieur-Technik
ISSN: 0009-286X
, E-ISSN: 1522-2640
|
| Output data |
Year: 2014,
Volume: 86,
Number: 11,
Pages: 1855-1870
Pages count
: 16
DOI:
10.1002/cite.201400068
|
| Tags |
Methane, Oxidative coupling, Process intensification, Reforming |
| Authors |
Thybaut Joris W.
1
,
Marin Guy B.
1
,
Mirodatos Claude
2
,
Schuurman Yves
2
,
van Veen Andre C.
3
,
Sadykov Vladislav A.
4,5
,
Pennemann Helmut
6
,
Bellinghausen Rainer
7
,
Mleczko Leslaw
7
|
| Affiliations |
| 1 |
Ghent University, Laboratory for Chemical Technology, Technologiepark-Zwijnaarde 914, 9052 Ghent, Belgium
|
| 2 |
Institutde Recherches sur la Catalyse et l’Environnement de Lyon (CNRS), 2 avenue Albert Einstein, 69626 Villeurbanne cedex, Lyon, France
|
| 3 |
Ruhr-Universität Bochum, Lehrstuhl für Technische Chemie, Universitätsstraße 150, 44801 Bochum, Germany
|
| 4 |
Novosibirsk State University
|
| 5 |
Boreskov Institute of Catalysis, Pr. akademika Lavrentieva 5, Novosibirsk 630090, Russia
|
| 6 |
Fraunhofer ICT-IMM, Carl-Zeiss-Straße 18 – 20, 55129 Mainz, Germany
|
| 7 |
Bayer Technology Services GmbH, BTS-TD-UP-CRT, Building E41, 51368 Leverkusen, Germany
|
|
A novel process concept for the oxidative coupling of methane followed by the oligomerization to liquids has been developed within the frame of the EU integrated project OCMOL. This technology is based on process intensification principles via cutting-edge structured microreactor technology. It is also a fully integrated industrial process through the re-use and the recycling of by-products, in particular CO2, at every process stage. The focus of this contribution is on the reaction engineering aspects of the core steps, i.e., catalysts, kinetics and reactor design for the methane coupling and reforming