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A Novel Technology for Natural Gas Conversion by Means of Integrated Oxidative Coupling and Dry Reforming of Methane Review

Общее Language: Английский, Genre: Review,
Status: Published, Source type: Original
Journal Chemie-Ingenieur-Technik
ISSN: 0009-286X , E-ISSN: 1522-2640
Output data Year: 2014, Volume: 86, Number: 11, Pages: 1855-1870 Pages count : 16 DOI: 10.1002/cite.201400068
Tags Methane, Oxidative coupling, Process intensification, Reforming
Authors Thybaut Joris W. 1 , Marin Guy B. 1 , Mirodatos Claude 2 , Schuurman Yves 2 , van Veen Andre C. 3 , Sadykov Vladislav A. 4,5 , Pennemann Helmut 6 , Bellinghausen Rainer 7 , Mleczko Leslaw 7
Affiliations
1 Ghent University, Laboratory for Chemical Technology, Technologiepark-Zwijnaarde 914, 9052 Ghent, Belgium
2 Institutde Recherches sur la Catalyse et l’Environnement de Lyon (CNRS), 2 avenue Albert Einstein, 69626 Villeurbanne cedex, Lyon, France
3 Ruhr-Universität Bochum, Lehrstuhl für Technische Chemie, Universitätsstraße 150, 44801 Bochum, Germany
4 Novosibirsk State University
5 Boreskov Institute of Catalysis, Pr. akademika Lavrentieva 5, Novosibirsk 630090, Russia
6 Fraunhofer ICT-IMM, Carl-Zeiss-Straße 18 – 20, 55129 Mainz, Germany
7 Bayer Technology Services GmbH, BTS-TD-UP-CRT, Building E41, 51368 Leverkusen, Germany

Abstract: A novel process concept for the oxidative coupling of methane followed by the oligomerization to liquids has been developed within the frame of the EU integrated project OCMOL. This technology is based on process intensification principles via cutting-edge structured microreactor technology. It is also a fully integrated industrial process through the re-use and the recycling of by-products, in particular CO2, at every process stage. The focus of this contribution is on the reaction engineering aspects of the core steps, i.e., catalysts, kinetics and reactor design for the methane coupling and reforming
Cite: Thybaut J.W. , Marin G.B. , Mirodatos C. , Schuurman Y. , van Veen A.C. , Sadykov V.A. , Pennemann H. , Bellinghausen R. , Mleczko L.
A Novel Technology for Natural Gas Conversion by Means of Integrated Oxidative Coupling and Dry Reforming of Methane
Chemie-Ingenieur-Technik. 2014. V.86. N11. P.1855-1870. DOI: 10.1002/cite.201400068 publication_identifier_short.wos_identifier_type publication_identifier_short.scopus_identifier_type publication_identifier_short.rinz_identifier_type
Dates:
Submitted: May 2, 2014
Accepted: Aug 22, 2014
Published online: Oct 10, 2014
Published print: Nov 1, 2014
Identifiers:
publication_identifier.wos_identifier_type WOS:000344249200002
publication_identifier.scopus_identifier_type 2-s2.0-84911932035
publication_identifier.rinz_identifier_type 24006933
publication_identifier.accession_number_identifier_type 2014:1779852
publication_identifier.chemical_accession_number_identifier_type 163:147969
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