Laser-Assisted Preparation of Highly-Efficient Photocatalytic Nanomaterial Based on Bismuth Silicate
Научная публикация
| Общая информация |
Язык:
Английский,
Жанр:
Статья (Full article),
Статус опубликования:
Опубликована,
Оригинальность:
Оригинальная
|
| Журнал |
Applied Surface Science
ISSN: 0169-4332
|
| Вых. Данные |
Год: 2022,
Том: 575,
Номер статьи
: 151732,
Страниц
: 12
DOI:
10.1016/j.apsusc.2021.151732
|
| Ключевые слова |
Bismuth silicate; Laser ablation in liquid phase; Laser irradiation of colloids; Nanoparticles; Photocatalysis |
| Авторы |
Shabalina A.V.
1
,
Fakhrutdinova E.D.
1
,
Golubovskaya A.G.
1
,
Kuzmin S.M.
2
,
Koscheev S.V.
3
,
Kulinich S.A.
4,5
,
Svetlichnyi V.A.
1
,
Vodyankina O.V.
1
|
| Организации |
| 1 |
Tomsk State University, Tomsk 634050, Russian Federation
|
| 2 |
G.A. Krestov Institute of Solution Chemistry of the Russian Academy of Sciences, Ivanovo 153045, Russian Federation
|
| 3 |
Boreskov Institute of Catalysis SB RAS, Novosibirsk, 630090, Russian Federation
|
| 4 |
Tokai University, Research Institute of Science and Technology, Hiratsuka, Kanagawa 259-1292, Japan
|
| 5 |
Far Eastern Federal University, Vladivostok 690091, Russian Federation
|
|
Информация о финансировании (1)
|
1
|
Российский научный фонд
|
19-73-30026 (АААА-А19-119052990037-6)
|
Having a wide range of applications, bismuth silicate-based materials (BSO) attract attention of numerous researchers. Typically, they are synthesized either from active chemicals or through high-energy impact on their precursors. The present work is the first report on BSO-based nanomaterials prepared via laser processing in liquid phase in which the following two-step scheme was realized: (1) Individual colloids of Bi- and Si-based nanoparticles were obtained via ablating their metallic targets in distilled water and then mixed; (2) Post-treatment of the mixed colloid was performed with the same laser beam as in stage (1). The products obtained after drying of non-treated and post-treated mixed colloids (denoted as samples BSO and BSO_hν, respectively) were carefully characterized using a set of microscopic, spectroscopic and electrochemical analyses, after which their photocatalytic performance in presence of model organic dye (rhodamine B) and phenol was tested. The additional laser treatment was found to lead to active interaction between Bi- and Si-containing species and stimulated formation of phases with Bi-O-Si bonds. The post-irradiated sample BSO_hν showed improved stability and catalytic performance, thus opening avenues for wider use of laser processing in liquids as a method allowing for preparation of nanostructures with complex chemical composition. © 2021 Elsevier B.V.