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Homogeneous High-Temperature Oxidation of Methane Научная публикация

Журнал Reaction Kinetics and Catalysis Letters
ISSN: 0133-1736 , E-ISSN: 1588-2837
Вых. Данные Год: 2007, Том: 91, Номер: 2, Страницы: 273-282 Страниц : 10 DOI: 10.1007/s11144-007-5158-5
Ключевые слова Homogeneous reactions, Kinetics, Lean mixtures, Methane oxidation
Авторы Slepterev Artem A. 1 , Salnikov Valerii S. 1 , Tsyrulnikov Pavel G. 1 , Noskov Aleksandr S. 2 , Tomilov Viktor N. 2 , Chumakova Nataliya A. 2 , Zagoruiko Andrey N. 2
Организации
1 Institute of Hydrocarbon Processing SB RAS, Neftezavodskaya str., 54, 644040 Omsk, Russia
2 Boreskov Institute of Catalysis SB RAS, Pr. Аkad. Lavrentieva 5, 630090 Novosibirsk, Russia

Информация о финансировании (1)

1 European Commission INCO-COPERNICUS ICA2-CT-2000-10035

Реферат: The kinetics of homogeneous deep oxidation of methane in lean mixtures (up to 2 vol % CH4 in air) in ceramic tubes and fixed beds of ceramic spheres was studied. Experiments with the homogeneous reaction have shown that the methane oxidation occurs via a consecutive scheme through CO formation. The reaction rate of CH4 oxidation was found to depend upon the equivalent pass diameter with a significant reaction inhibition in packing of small tubes and spheres, reflecting the influence of mass transfer on the radical-chain termination at the ceramic surfaces. It was also found that CO oxidation practically does not depend upon the mass exchange conditions, but it is visibly inhibited by methane. Recommended kinetic equations and their parameters are presented.
Библиографическая ссылка: Slepterev A.A. , Salnikov V.S. , Tsyrulnikov P.G. , Noskov A.S. , Tomilov V.N. , Chumakova N.A. , Zagoruiko A.N.
Homogeneous High-Temperature Oxidation of Methane
Reaction Kinetics and Catalysis Letters. 2007. V.91. N2. P.273-282. DOI: 10.1007/s11144-007-5158-5 WOS Scopus РИНЦ CAPlusCA OpenAlex
Даты:
Поступила в редакцию: 17 мая 2007 г.
Принята к публикации: 24 мая 2007 г.
Опубликована online: 12 авг. 2007 г.
Опубликована в печати: 1 сент. 2007 г.
Идентификаторы БД:
Web of science: WOS:000248818700010
Scopus: 2-s2.0-34547903828
РИНЦ: 13549230
Chemical Abstracts: 2007:898320
Chemical Abstracts (print): 150:194958
OpenAlex: W1971229526
Цитирование в БД:
БД Цитирований
Web of science 17
Scopus 20
РИНЦ 21
OpenAlex 21
Альметрики: