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Modeling of a Heat-Integrated Catalytic Reformer/Combustor of Methane: Fine Balancing between Hot Spots and Extinction Научная публикация

Журнал Chemical Engineering and Technology
ISSN: 0930-7516 , E-ISSN: 1521-4125
Вых. Данные Год: 2009, Том: 32, Номер: 9, Страницы: 1367-1375 Страниц : 9 DOI: 10.1002/ceat.200900197
Ключевые слова Endothermic reactions, Exothermic reactions, Heat integration, Hydrogen production, Methane combustion, Methane steam reforming, Parametric sensitivity hysteresis, Reactor modeling
Авторы Shigarov Alexey B. 1 , Fadeev Stanislav I. 2 , Kirillov Valery A. 1
Организации
1 Boreskov Institute of Catalysis, Novosibirsk, Russia
2 Sobolev Institute of Mathematics, Novosibirsk, Russia

Информация о финансировании (1)

1 Международный научно-технический центр 2904

Реферат: Modeling is used to study the parametric sensitivity of a heat-integrated methane steam reformer/combustor for hydrogen production. The simulated reformer design is based on structured metal-porous catalysts and the co-current flow mode operation. The modeling results indicate that the reformer has high intrinsic sensitivity to the kinetic activity of reforming and combustion catalysts and to the axial or transversal coefficients of heat conductivity. Moreover, a hysteresis effect with critical points of ignition and extinction was found under synchronous load variation in the reforming and combustion units. These results show that fine tuning of the main design parameters is necessary to avoid both hot spot formation and extinction.
Библиографическая ссылка: Shigarov A.B. , Fadeev S.I. , Kirillov V.A.
Modeling of a Heat-Integrated Catalytic Reformer/Combustor of Methane: Fine Balancing between Hot Spots and Extinction
Chemical Engineering and Technology. 2009. V.32. N9. P.1367-1375. DOI: 10.1002/ceat.200900197 WOS Scopus РИНЦ CAPlusCA OpenAlex
Даты:
Принята к публикации: 2 февр. 2009 г.
Поступила в редакцию: 17 апр. 2009 г.
Опубликована online: 7 авг. 2009 г.
Опубликована в печати: 1 сент. 2009 г.
Идентификаторы БД:
Web of science: WOS:000269766700010
Scopus: 2-s2.0-69949120633
РИНЦ: 15310986
Chemical Abstracts: 2009:1068182
Chemical Abstracts (print): 153:149689
OpenAlex: W2079539913
Цитирование в БД:
БД Цитирований
Web of science 14
Scopus 14
РИНЦ 11
OpenAlex 15
Альметрики: