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Low-Temperature Fabrication of SiOx-TiO2 Core-Shell Nanowires for Photocatalytic Application Full article

Journal Vacuum
ISSN: 0042-207X
Output data Year: 2019, Volume: 165, Pages: 51-57 Pages count : 7 DOI: 10.1016/j.vacuum.2019.03.059
Tags Silicon oxide nanowires, Core-shell structure, Atomic layer deposition, TiO2 photocatalyst
Authors Lebedev M.S. 1 , Khmel S.Ya. 2 , Lyulyukin M.N. 3,4 , Petukhova D.E. 1,4 , Barsukov A.V. 4
Affiliations
1 Nikolaev Institute of Inorganic Chemistry SB RAS
2 Kutateladze Institute of Thermophysics SB RAS
3 Boreskov Institute of Catalysis SB RAS
4 Novosibirsk State University

Funding (1)

1 Federal Agency for Scientific Organizations V.45.1.5

Abstract: A new low-temperature fabrication method of SiOx-TiO2 core-shell nanowires (NWs) for photocatalytic application was suggested. In the present work, the gas-jet electron beam plasma chemical vapor deposition method was used to synthesize arrays of oriented bundles (microropes) of silicon oxide NWs. Tin nanoparticles were used as catalyst for the NW growth via the “vapor-liquid-solid” mechanism at a temperature of 335 °C. A conformal nanocrystalline TiO2 coating was then deposited by atomic layer deposition using TiCl4 and H2O at 300 °C. Anatase phase formation was confirmed by Raman spectroscopy and X-ray diffraction. The photocatalytic characteristics of the fabricated arrays were demonstrated by the example of the photo-oxidation reaction of acetone vapor. Options for further development and advantages of the method such as low temperature, scalability and good compatibility of the fabrication stages are discussed.
Cite: Lebedev M.S. , Khmel S.Y. , Lyulyukin M.N. , Petukhova D.E. , Barsukov A.V.
Low-Temperature Fabrication of SiOx-TiO2 Core-Shell Nanowires for Photocatalytic Application
Vacuum. 2019. V.165. P.51-57. DOI: 10.1016/j.vacuum.2019.03.059 WOS Scopus РИНЦ AN OpenAlex
Dates:
Submitted: Mar 10, 2019
Accepted: Mar 30, 2019
Published online: Apr 5, 2019
Published print: Jul 1, 2019
Identifiers:
Web of science: WOS:000470047600008
Scopus: 2-s2.0-85064068192
Elibrary: 38688663
Chemical Abstracts: 2019:736103
OpenAlex: W2929605568
Citing:
DB Citing
Scopus 9
Web of science 7
Elibrary 10
OpenAlex 7
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