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Thermally Coupled Catalytic Reactor for Steam Reforming of Methane and Liquid Hydrocarbons: Experiment and Mathematical Modeling Full article

Journal Theoretical Foundations of Chemical Engineering
ISSN: 0040-5795 , E-ISSN: 1608-3431
Output data Year: 2003, Volume: 37, Number: 3, Pages: 276-284 Pages count : 9 DOI: 10.1023/A:1024039823317
Tags Methane; Steam; Catalytic Reactor; Reaction Zone; Thermal Condition
Authors Kirillov V.A. 1 , Kuzin N.A. 1 , Kulikov A.V. 1 , Fadeev S.I. 2 , Shigarov A.B. 1 , Sobyanin V.A. 1
Affiliations
1 Boreskov Institute of Catalysis, Siberian Division, Russian Academy of Sciences, pr. Akademika Lavrent’eva 5, Novosibirsk, 630090 Russia
2 Sobolev Institute of Mathematics, Siberian Division, Russian Academy of Sciences, pr. Akademika Koptyuga 4, Novosibirsk, 630090 Russia

Funding (1)

1 International Science and Technology Center 2291

Abstract: An energy-efficient catalytic reactor for producing synthesis gas from methane and liquid hydrocarbons is proposed that is based on the coupling of an endothermic reaction (steam reforming of methane, hexane, or isooctane) and an exothermic reaction (hydrogen oxidation by atmospheric oxygen) in a single cocurrent apparatus. To describe the processes in such an apparatus, a two-dimensional two-temperature mathematical model is developed. It was revealed experimentally and by mathematical modeling that the heat- and mass-transfer coefficients of the gas flow in contact with the catalytically active wall in the exothermic reaction zone considerably affect the thermal conditions in the reactor.
Cite: Kirillov V.A. , Kuzin N.A. , Kulikov A.V. , Fadeev S.I. , Shigarov A.B. , Sobyanin V.A.
Thermally Coupled Catalytic Reactor for Steam Reforming of Methane and Liquid Hydrocarbons: Experiment and Mathematical Modeling
Theoretical Foundations of Chemical Engineering. 2003. V.37. N3. P.276-284. DOI: 10.1023/A:1024039823317 WOS Scopus РИНЦ ANCAN OpenAlex
Original: Кириллов В.А. , Кузин Н.А. , Куликов А.В. , Фадеев С.И. , Шигаров А.Б. , Собянин В.А.
Сопряженный по тепловым потокам каталитический реактор паровой конверсии метана и жидких углеводородов. Эксперимент и математическое моделирование.
Теоретические основы химической технологии. 2003. Т.37. №3. С.300-308. Scopus РИНЦ
Dates:
Submitted: Aug 30, 2002
Published print: May 1, 2003
Identifiers:
Web of science: WOS:000183780100011
Scopus: 2-s2.0-0038542090
Elibrary: 13440048
Chemical Abstracts: 2003:432519
Chemical Abstracts (print): 139:232720
OpenAlex: W251007168
Citing:
DB Citing
Web of science 16
Scopus 21
Elibrary 19
OpenAlex 22
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