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Two-Component Model for Catalyst Deactivation Научная публикация

Журнал Chemical Engineering Journal
ISSN: 1385-8947 , E-ISSN: 1873-3212
Вых. Данные Год: 2019, Том: 378, Номер статьи : 122176, Страниц : 4 DOI: 10.1016/j.cej.2019.122176
Ключевые слова Catalyst deactivation; Fick's law; Non-homogeneous model
Авторы Malkovich E.G. 1,2 , Parkhomchuk E.V. 2,3 , Bazaikin Ya.V. 1,2 , Lysikov A.I. 2,3
Организации
1 Sobolev Institute of Mathematics SB RAS, Novosibirsk, Russian Federation
2 Novosibirsk State University, Novosibirsk, Russian Federation
3 Boreskov Institute of Catalysis SB RAS, Novosibirsk, Russian Federation

Информация о финансировании (2)

1 Российский фонд фундаментальных исследований 17-43-543303 (АААА-А17-117062810020-4)
2 Министерство науки и высшего образования Российской Федерации (с 15 мая 2018) 0314-2019-0006 (АААА-А19-119021890014-4)

Реферат: Texture evolution of alumina hydrotreating catalyst was theoretically modeled using geometrical characteristics calculated via Monte-Carlo methods and methods of the graph theory. In the prescribed model deactivation was specified by monotonic increase of alumina grain radius, which imitated deposition of coke and metal species onto the pore surface. A novel two-component nonhomogeneous model was designed based on the diffusion of asphaltene molecules inside the cylindrical pellet according to Fick's law and deposition of the coke particles from heavy oil on the surface of the catalyst. The model resulted in non-monotonous coke distribution with a distinct maximum in the inner region of the pellet, which, nevertheless, shifts to the center at later deactivation stages due to the higher hydrogenation performance of pellet border region. Model can be applied to describe profiles of coke depositions during deactivation process for a pellet with an arbitrary boundary. © 2019 Elsevier B.V.
Библиографическая ссылка: Malkovich E.G. , Parkhomchuk E.V. , Bazaikin Y.V. , Lysikov A.I.
Two-Component Model for Catalyst Deactivation
Chemical Engineering Journal. 2019. V.378. 122176 :1-4. DOI: 10.1016/j.cej.2019.122176 WOS Scopus РИНЦ CAPlusCA OpenAlex
Даты:
Опубликована online: 8 июл. 2019 г.
Опубликована в печати: 15 дек. 2019 г.
Идентификаторы БД:
Web of science: WOS:000487764800105
Scopus: 2-s2.0-85069551312
РИНЦ: 41619868
Chemical Abstracts: 2019:1412968
Chemical Abstracts (print): 171:240917
OpenAlex: W2957720902
Цитирование в БД:
БД Цитирований
Scopus 8
Web of science 8
РИНЦ 6
OpenAlex 9
Альметрики: