Influence of a Reaction Mixture Streamline on Partial Oxidation of Methane in an Asymmetric Microchannel Reactor | Sciact - CRIS-system of Boreskov Institute of Catalysis

Influence of a Reaction Mixture Streamline on Partial Oxidation of Methane in an Asymmetric Microchannel Reactor Full article

Journal

International Journal of Hydrogen Energy
ISSN: 0360-3199 , E-ISSN: 1879-3487

Output data

Year: 2014, Volume: 39, Number: 1, Pages: 325-330 Pages count : 6 DOI: 10.1016/j.ijhydene.2013.10.040

Tags

Catalytic microreactor, Hydrogen production, Microchannel plate, Partial oxidation of methane, Syngas

Authors

Vorontsov V.A. ¹ , Gribovskiy A.G. ^2,3 , Makarshin L.L. ³ , Andreev D.V. ³ , Ylianitsky V.Y. ⁴ , Parmon V.N. ^2,3

Affiliations

1	Novosibirsk State Technical University, Pr. K. Marksa 20, 630073 Novosibirsk, Russia
2	Novosibirsk State University, ul. Pirogova 2, 630090 Novosibirsk, Russia
3	Boreskov Institute of Catalysis, Pr. Akad. Lavrentieva 5, 630090 Novosibirsk, Russia
4	Lavrentiev Institute of Hydrodynamics, Pr. Akad. Lavrentieva 15, 630090 Novosibirsk, Russia

Funding (1)

Russian Foundation for Basic Research

13-08-00449

Partial oxidation of methane (POM) has been tested in an asymmetric microchannel reactor with different inlet configurations. One inlet of the reactor provided successive splitting of an inlet flow into parallel channels, whereas the opposite inlet allowed the inlet flow to enter the parallel channels simultaneously. It was found that concentrations of carbon monoxide and carbon dioxide changed by 20–30% and the conversion of methane changed by 5–20%, depending on the rate and direction of the inlet flow. The hydrogen production rate practically did not depend on the inlet configuration and equaled 15 l/h at the inlet flow rates from 600 to 1400 cm3/min and at the methane conversion of 80%. The data obtained demonstrated that the use of different operating modes of the asymmetric microreactor allows changing the composition of produced syngas.

Vorontsov V.A. , Gribovskiy A.G. , Makarshin L.L. , Andreev D.V. , Ylianitsky V.Y. , Parmon V.N.
Influence of a Reaction Mixture Streamline on Partial Oxidation of Methane in an Asymmetric Microchannel Reactor
International Journal of Hydrogen Energy. 2014. V.39. N1. P.325-330. DOI: 10.1016/j.ijhydene.2013.10.040 WOS Scopus РИНЦ ANCAN OpenAlex

Submitted:	Jun 11, 2013
Accepted:	Oct 7, 2013
Published online:	Nov 7, 2013
Published print:	Jan 2, 2014

Web of science:	WOS:000330921800032
Scopus:	2-s2.0-84890383939
Elibrary:	21861910
Chemical Abstracts:	2013:1744548
Chemical Abstracts (print):	160:251438
OpenAlex:	W2045607728

DB	Citing
Web of science	7
Scopus	8
Elibrary	8
OpenAlex	9