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Effect of Asymmetric Membrane Structure on Hydrogen Transport Resistance and Performance of a Catalytic Membrane Reactor for Ethanol Steam Reforming Научная публикация

Журнал Membranes
ISSN: 2077-0375
Вых. Данные Год: 2021, Том: 11, Номер: 5, Номер статьи : 332, Страниц : 29 DOI: 10.3390/membranes11050332
Ключевые слова membrane reactor modeling; ethanol steam reforming; asymmetric supported membrane
Авторы Bobrova Ludmilla 1 , Eremeev Nikita 1 , Vernikovskaya Nadezhda 1 , Sadykov Vladislav 1,2 , Smorygo Oleg 3
Организации
1 Federal Research Center, Boreskov Institute of Catalysis SB RAS, 630090 Novosibirsk, Russia
2 Department of Physics, Novosibirsk State University, 630090 Novosibirsk, Russia
3 O.V. Roman Powder Metallurgy Institute, 220005 Minsk, Belarus

Информация о финансировании (2)

1 Министерство науки и высшего образования Российской Федерации (с 15 мая 2018) 0239-2021-0005
2 Министерство науки и высшего образования Российской Федерации (с 15 мая 2018) 0239-2021-0011

Реферат: The performance of catalytic membrane reactors (CMRs) depends on the specific details of interactions at different levels between catalytic and separation parts. A clear understanding of decisive factors affecting their operational parameters can be provided via mathematical simulations. In the present paper, main results of numerical studies of ethanol steam reforming, followed by downstream hydrogen permeation through an asymmetric supported membrane, are reported. The membrane module consists of a thin selective layer supported on a substrate with graded porous structure. One-dimensional isothermal reaction–transport model for the CMR has been developed, and its validation has been carried out by using performance data from a lab-scale reactor with a disk-shaped membrane. Simulations demonstrate the model’s capabilities to analyze local concentrations gradients, as required to provide accurate estimates of the relationship between structure–property–performance. It was shown that transport properties of multilayer asymmetric membranes are highly related to the structural properties of each single layer.
Библиографическая ссылка: Bobrova L. , Eremeev N. , Vernikovskaya N. , Sadykov V. , Smorygo O.
Effect of Asymmetric Membrane Structure on Hydrogen Transport Resistance and Performance of a Catalytic Membrane Reactor for Ethanol Steam Reforming
Membranes. 2021. V.11. N5. 332 :1-29. DOI: 10.3390/membranes11050332 WOS Scopus РИНЦ CAPlus PMID OpenAlex
Файлы: Полный текст от издателя
Даты:
Поступила в редакцию: 11 апр. 2021 г.
Принята к публикации: 27 апр. 2021 г.
Опубликована online: 30 апр. 2021 г.
Опубликована в печати: 1 мая 2021 г.
Идентификаторы БД:
Web of science: WOS:000654308800001
Scopus: 2-s2.0-85105584614
РИНЦ: 46089151
Chemical Abstracts: 2021:1340677
PMID (PubMed): 33946242
OpenAlex: W3158959759
Цитирование в БД:
БД Цитирований
Scopus 7
Web of science 7
РИНЦ 8
OpenAlex 7
Альметрики: