Element Selective Magnetism in Ho0.5Nd0.5Fe3(BO3)4 Single Crystal Probed with Hard X-ray Magnetic Circular Dichroism Full article
Journal |
Journal of Magnetism and Magnetic Materials
ISSN: 0304-8853 |
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Output data | Year: 2019, Volume: 479, Pages: 312-316 Pages count : 5 DOI: 10.1016/j.jmmm.2019.02.040 | ||||||||
Tags | X-ray magnetic circular dichroism; X-ray absorption; Magnetic properties | ||||||||
Authors |
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Affiliations |
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Abstract:
We present a study of a Ho0.5Nd0.5Fe3(BO3)(4) single crystal aiming at understanding the roles of each magnetic sublattices in magnetic transitions at low temperatures. The crystal structure is determined to have the R32 symmetry in whole studied temperature range but the crystal appears to be racemic. Element selective magnetic properties studied with X-ray magnetic circular dichroism at the L-2,L-3-edges of Ho and Nd, and at the Fe K-edge at T = 3 K under magnetic fields of +/- 17 T are compared with the results of macroscopic magnetization measurements in pure and substituted crystals. All three magnetic sublattices are shown to be strongly coupled and to undergo a spin-reorientation transition when magnetic field is applied along the trigonal c-axis. On the contrary, when magnetic field is applied in the ab-plane only the holmium atoms exhibit a sizeable magnetization jump. This result allows us to conclude that the spin-flop transitions observed in macroscopic magnetization curves and associated anomalies of electric polarization are due to the Ho3+ magnetic moment reorientation.
Cite:
Platunov M.
, Kazak N.
, Dudnikov V.
, Temerov V.
, Gudim I.
, Knyazev Y.
, Gavrilkin S.
, Dyadkin V.
, Dovgaliuk I.
, Chernyshov D.
, Hen A.
, Wilhelm F.
, Rogalev A.
, Ovchinnikov S.
Element Selective Magnetism in Ho0.5Nd0.5Fe3(BO3)4 Single Crystal Probed with Hard X-ray Magnetic Circular Dichroism
Journal of Magnetism and Magnetic Materials. 2019. V.479. P.312-316. DOI: 10.1016/j.jmmm.2019.02.040 WOS Scopus РИНЦ ANCAN OpenAlex
Element Selective Magnetism in Ho0.5Nd0.5Fe3(BO3)4 Single Crystal Probed with Hard X-ray Magnetic Circular Dichroism
Journal of Magnetism and Magnetic Materials. 2019. V.479. P.312-316. DOI: 10.1016/j.jmmm.2019.02.040 WOS Scopus РИНЦ ANCAN OpenAlex
Dates:
Submitted: | Nov 26, 2018 |
Accepted: | Feb 14, 2019 |
Published online: | Feb 14, 2019 |
Published print: | Jun 1, 2019 |
Identifiers:
Web of science: | WOS:000459863200047 |
Scopus: | 2-s2.0-85061832213 |
Elibrary: | 38644400 |
Chemical Abstracts: | 2019:350542 |
Chemical Abstracts (print): | 170:474594 |
OpenAlex: | W2914077098 |