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Simulation of Hydrogen and Propylene Coproduction in Catalytic Membrane Reactor Full article

Journal International Journal of Hydrogen Energy
ISSN: 0360-3199 , E-ISSN: 1879-3487
Output data Year: 2015, Volume: 40, Number: 8, Pages: 3592-3598 Pages count : 7 DOI: 10.1016/j.ijhydene.2014.09.004
Tags Alkane dehydrogenation, Hydrogen production, Membrane reactor, Pore size distribution, Porous ceramic membrane
Authors Shelepova E.V. 1 , Vedyagin A.A. 1,2 , Mishakov I.V. 1,2 , Noskov A.S. 1,2
Affiliations
1 Boreskov Institute of Catalysis, Siberian Branch, Russian Academy of Sciences, 5 pr. Lavrentieva, Novosibirsk 630090, Russia
2 Novosibirsk State Technical University, 20 pr. Marksa, Novosibirsk 630073, Russia

Abstract: A two-dimensional non isothermal mathematical model has been developed to simulate the propane dehydrogenation in a catalytic membrane reactor with tube-and-shell configuration. The permeable inner tube consists of an inert large-pore support and thin microporous membrane layer. The membrane removes hydrogen from reaction zone shifting the reaction equilibrium towards products. Both pores diameter and membrane thickness were varied to obtain the optimal membrane characteristics in terms of hydrogen and propylene productivity, and hydrogen purity. The model correctly predicted the improved process parameters when the membrane thickness was 4 μm and the pore diameter was 0.4 nm.
Cite: Shelepova E.V. , Vedyagin A.A. , Mishakov I.V. , Noskov A.S.
Simulation of Hydrogen and Propylene Coproduction in Catalytic Membrane Reactor
International Journal of Hydrogen Energy. 2015. V.40. N8. P.3592-3598. DOI: 10.1016/j.ijhydene.2014.09.004 WOS Scopus РИНЦ ANCAN OpenAlex
Dates:
Submitted: Jun 6, 2014
Accepted: Sep 2, 2014
Published online: Sep 26, 2014
Published print: Mar 1, 2015
Identifiers:
Web of science: WOS:000350939600049
Scopus: 2-s2.0-84922876546
Elibrary: 24008321
Chemical Abstracts: 2014:1601574
Chemical Abstracts (print): 162:258801
OpenAlex: W2002516653
Citing:
DB Citing
Web of science 30
Scopus 30
Elibrary 27
OpenAlex 32
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