XMCD and ab-initio Study of Interface-Engineered Ultrathin Ru/Co/W/Ru Films with Perpendicular Magnetic Anisotropy and Strong Dzyaloshinskii-Moriya Interaction | Sciact - CRIS-system of Boreskov Institute of Catalysis

XMCD and ab-initio Study of Interface-Engineered Ultrathin Ru/Co/W/Ru Films with Perpendicular Magnetic Anisotropy and Strong Dzyaloshinskii-Moriya Interaction Full article

Journal

PCCP: Physical Chemistry Chemical Physics
ISSN: 1463-9076 , E-ISSN: 1463-9084

Output data

Year: 2022, Volume: 24, Pages: 8225-8232 Pages count : 7 DOI: 10.1039/D1CP05456B

Tags

TOTAL-ENERGY CALCULATIONS; CIRCULAR-DICHROISM; MOLECULAR-DYNAMICS; K-EDGE; COTRANSITION; SCATTERING

Authors

Samardak Alexander S. ¹ , Ognev Alexey V. ¹ , Kolesnikov Alexander G. ¹ , Stebliy Maksim E. ¹ , Samardak Vadim Yu. ¹ , Iliushin Ilia G. ¹ , Pervishko Anastasiia A. ² , Yudin Dmitry ² , Platunov Mikhail ^3,4 , Ono Teruo ^1,5 , Wilhelm Fabrice ⁶ , Rogalev Andrey ⁶

Affiliations

1	Institute of High Technologies and Advanced Materials, Far Eastern Federal University, 690922 Vladivostok, Russia
2	Skolkovo Institute of Science and Technology, 121205 Moscow, Russia
3	Kirensky Institute of Physics, Federal Research Center KSC SB RAS, 660036 Krasnoyarsk, Russia.
4	Synchrotron radiation facility SKIF, Boreskov Institute of Catalysis SB RAS, 630559 Kol’tsovo, Russia
5	Institute for Chemical Research, Kyoto University, Uji, Kyoto, Japan
6	ESRF-The European Synchrotron, 38043 Grenoble Cedex 9, France

Funding (5)

1	Ministry of Science and Higher Education of the Russian Federation	ГЗ-2021-2023
2	Ministry of Science and Higher Education of the Russian Federation	075-15-2021-607
3	Ministry of Science and Higher Education of the Russian Federation	0657-2020-0013 (221042200121-9)
4	Russian Foundation for Basic Research	19-32-60020 (АААА-А19-119111590033-6)
5	Russian Science Foundation	21-42-00041 (121051700022-7)

Understanding the nature of recently discovered spin-orbital induced phenomena and a definition of a general approach for “ferromagnet/heavy-metal” layered systems to enhance and manipulate spin-orbit coupling, spin-orbit torque, and the Dzyaloshinskii-Moriya interaction (DMI) assisted by atomic-scale interface engineering are essential for developing spintronics and spin-orbitronics. Here, we exploit X-ray magnetic circular dichroism (XMCD) spectroscopy at the L2,3-edges of 5d and 4d non-magnetic heavy metals (W and Ru, respectively) in ultrathin Ru/Co/W/Ru films to determine their induced magnetic moments due to the proximity to the ferromagnetic layer of Co. The deduced orbital and spin magnetic moments agree well with the theoretically predicted values, highlighting the drastic effect of constituting layers on the system’s magnetic properties and the strong interfacial DMI in Ru/Co/W/Ru films. As a result, we demonstrate the ability to simultaneously control the strength of magnetic anisotropy and intermixing-enhanced DMI through the interface engineered inversion asymmetry in the thin-film chiral ferromagnets, which are a potential host for stable magnetic skyrmions.

Samardak A.S. , Ognev A.V. , Kolesnikov A.G. , Stebliy M.E. , Samardak V.Y. , Iliushin I.G. , Pervishko A.A. , Yudin D. , Platunov M. , Ono T. , Wilhelm F. , Rogalev A.
XMCD and ab-initio Study of Interface-Engineered Ultrathin Ru/Co/W/Ru Films with Perpendicular Magnetic Anisotropy and Strong Dzyaloshinskii-Moriya Interaction
PCCP: Physical Chemistry Chemical Physics. 2022. V.24. P.8225-8232. DOI: 10.1039/D1CP05456B WOS Scopus РИНЦ ANCAN PMID OpenAlex publication_identifier_short.sciact_skif_identifier_type

Submitted:	Nov 30, 2021
Accepted:	Mar 7, 2022
Published online:	Mar 8, 2022
Published print:	Apr 6, 2022

Web of science:	WOS:000772106100001
Scopus:	2-s2.0-85128141682
Elibrary:	48427965
Chemical Abstracts:	2022:774710
Chemical Abstracts (print):	180:305092
PMID:	35319030
OpenAlex:	W4220991335
publication_identifier.sciact_skif_identifier_type:	1883

DB	Citing
Web of science	3
Scopus	4
Elibrary	3
OpenAlex	5