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Mastering the Molecular Dynamics of a Bistable Molecule by Single Atom Manipulation Full article

Journal Physical Review Letters
ISSN: 0031-9007 , E-ISSN: 1079-7114
Output data Year: 2006, Volume: 97, Number: 21, Article number : 216103, Pages count : 4 DOI: 10.1103/PhysRevLett.97.216103
Tags Absorption; Atomic physics; Low temperature operations; Molecular dynamics; Probability density function; Scanning tunneling microscopy
Authors Martin M. 1 , Lastapis M. 1 , Riedel D. 1 , Dujardin G. 1 , Mamatkulov M. 2 , Stauffer L. 2 , Sonnet Ph. 2
Affiliations
1 Laboratoire de Photophysique Moléculaire, Bâtiment 210, Université Paris Sud, 91405 Orsay Cedex, France
2 Laboratoire de Physique et de Spectroscopie électronique, Université de Haute Alsace-CNRS UMR 7014, 4, rue des Frères Lumière, 68093 Mulhouse Cedex, France

Abstract: At low temperature (5 K), a single biphenyl molecule adsorbed on a Si(100) surface behaves as a bistable device which can be reversibly switched by electronic excitation with the scanning tunneling microscope tip. Density functional theory suggests that the biphenyl molecule is adsorbed with one dissociated hydrogen atom bonded to a neighbor surface silicon atom. By desorbing this hydrogen atom with the STM tip, the interaction of the molecule with the surface is modified such that it becomes transformed into a multistable device with four stable states having switching yields increased by almost 2 orders of magnitude
Cite: Martin M. , Lastapis M. , Riedel D. , Dujardin G. , Mamatkulov M. , Stauffer L. , Sonnet P.
Mastering the Molecular Dynamics of a Bistable Molecule by Single Atom Manipulation
Physical Review Letters. 2006. V.97. N21. 216103 :1-4. DOI: 10.1103/PhysRevLett.97.216103 WOS Scopus РИНЦ OpenAlex
Dates:
Submitted: Apr 5, 2006
Published online: Nov 21, 2006
Published print: Nov 24, 2006
Identifiers:
Web of science: WOS:000242219900025
Scopus: 2-s2.0-33751256871
Elibrary: 48209375
OpenAlex: W2055387261
Citing:
DB Citing
Web of science 41
Scopus 42
OpenAlex 49
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