Sorption-Enhanced Reforming of Bioethanol in Dual Fixed Bed Reactor for Continuous Hydrogen Production | Sciact - CRIS-система Института катализа

Sorption-Enhanced Reforming of Bioethanol in Dual Fixed Bed Reactor for Continuous Hydrogen Production Научная публикация

Конференция

Euro-mediterranean Hydrogen Technologies Conference (EmHyTeC2014)
09-12 дек. 2014 , Taormina

Журнал

International Journal of Hydrogen Energy
ISSN: 0360-3199 , E-ISSN: 1879-3487

Вых. Данные

Год: 2015, Том: 40, Номер: 42, Страницы: 14436-14444 Страниц : 9 DOI: 10.1016/j.ijhydene.2015.06.029

Ключевые слова

Adsorption, Carbon dioxide sorbent, High temperature pressure swing, Hydrogen production, Sorption-enhanced reforming

Авторы

Lysikov Anton ^1,2,3,4 , Derevschikov Vladimir ^1,2,3 , Okunev Alexey ^1,2

Организации

1	Boreskov Institute of Catalysis, pr. Lavrentieva 5, Novosibirsk, 630090, Russia
2	Novosibirsk State University, Pirogova str. 2, Novosibirsk, 630090, Russia
3	Research and Education Centre, NSU, Pirogova str. 2, Novosibirsk, 630090, Russia
4	Strategic Development Program “MRA-199”, Skolkovo Institute of Science and Technology, Novaya Street 100, Moscow, 143025, Russia

Информация о финансировании (3)

1	Российский фонд фундаментальных исследований	14-03-31731
2	Сколковский институт науки и технологий	199-MRA
3	Совет по грантам Президента Российской Федерации	СП-3164.2015.1

The sorption enhanced reforming (SER) of ethanol over an admixture of CaO sorbent and Ni reforming catalyst has been experimentally studied in a periodically operated dual fixed bed reactor. The optimal parameters for SER process were calculated from thermodynamic data. The experiment was carried out in cyclic mode; temperature swing adsorption and pressure swing adsorption (PSA) modes were used for periodic sorbent regeneration. It was shown that the continuous hydrogen production and the purity of hydrogen during the sorption-catalytic ethanol reforming maintained at the constant level and were 50 L/min and 97e99 vol.% respectively. The dual fixed bed SER reactor worked fine during 2 months on stream and more than 250 cycles. Both the sorbent and the catalyst maintained the sufficient activity during experiment. The obtained results suggest that sorption enhanced reforming may be a perspective approach for hydrogen production in fuel cell powered cogeneration systems.

Lysikov A. , Derevschikov V. , Okunev A.
Sorption-Enhanced Reforming of Bioethanol in Dual Fixed Bed Reactor for Continuous Hydrogen Production
International Journal of Hydrogen Energy. 2015. V.40. N42. P.14436-14444. DOI: 10.1016/j.ijhydene.2015.06.029 WOS Scopus РИНЦ CAPlusCA OpenAlex

Поступила в редакцию:	26 февр. 2015 г.
Принята к публикации:	5 июн. 2015 г.
Опубликована online:	29 июн. 2015 г.
Опубликована в печати:	1 нояб. 2015 г.

Web of science:	WOS:000364256300003
Scopus:	2-s2.0-84948710231
РИНЦ:	25168994
Chemical Abstracts:	2015:1077981
Chemical Abstracts (print):	163:506949
OpenAlex:	W1939669115

БД	Цитирований
Web of science	10
Scopus	13
РИНЦ	12
OpenAlex	13