Self-Ordered Nanoporous Lattice Formed by Chlorine Atoms on Au(111) | Sciact - CRIS-system of Boreskov Institute of Catalysis

Self-Ordered Nanoporous Lattice Formed by Chlorine Atoms on Au(111) Full article

Journal

Physical Review B, Condensed Matter and Materials Physics (up to 2016)
ISSN: 1098-0121 , E-ISSN: 1550-235X

Output data

Year: 2016, Volume: 93, Number: 4, Article number : 045432, Pages count : 8 DOI: 10.1103/PhysRevB.93.045432

Tags

SCANNING-TUNNELING-MICROSCOPY; INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; HERRINGBONE RECONSTRUCTION; ISLAND NUCLEATION; SURFACE CHLORIDE; SOLID-SURFACES; ADSORPTION; METALS

Authors

Cherkez V.V. ^1,2 , Zheltov V.V. ¹ , Didiot C. ² , Kierren B. ² , Fagot-Revurat Y. ² , Malterre D. ² , Andryushechkin B.V. ¹ , Zhidomirov G.M. ^1,3 , Eltsov K.N. ¹

Affiliations

1	International Joint Laboratory IMTAS, A. M. Prokhorov General Physics Institute, Russian Academy of Sciences, Vavilov str. 38, 119991 Moscow, Russia
2	International Joint Laboratory IMTAS, Institut Jean Lamour-UMR CNRS 7198-equipe 102, Departement Physique de la Matiere et des Materiaux, B.P 239 Universite H. Poincare-Nancy, 54506 Vandoeuvre les Nancy, France
3	G. K. Boreskov Institute of Catalysis, Siberian Branch of the Russian Academy of Sciences, Prospect Lavrentieva 5, 630090 Novosibirsk, Russia

Funding (2)

1	Russian Foundation for Basic Research	15-02-99542
2	Президиум РАН	39

A self-ordered nanoporous lattice formed by individual chlorine atoms on the Au(111) surface has been studied with low-temperature scanning tunneling microscopy, low-energy electron diffraction, and density functional theory calculations. We have found out that room-temperature adsorption of 0.09–0.30 monolayers of chlorine on Au(111) followed by cooling below 110 K results in the spontaneous formation of a nanoporous quasihexagonal structure with a periodicity of 25–38 Å depending on the initial chlorine coverage. The driving force of the superstructure formation is attributed to the substrate-mediated elastic interaction.

Cherkez V.V. , Zheltov V.V. , Didiot C. , Kierren B. , Fagot-Revurat Y. , Malterre D. , Andryushechkin B.V. , Zhidomirov G.M. , Eltsov K.N.
Self-Ordered Nanoporous Lattice Formed by Chlorine Atoms on Au(111)

Physical Review B, Condensed Matter and Materials Physics (up to 2016). 2016. V.93. N4. 045432 :1-8. DOI: 10.1103/PhysRevB.93.045432 WOS Scopus РИНЦ AN OpenAlex

Full text from publisher

Submitted:	Apr 8, 2015
Accepted:	Nov 11, 2015
Published print:	Jan 1, 2016
Published online:	Jan 28, 2016

Web of science:	WOS:000369227400008
Scopus:	2-s2.0-85000838027
Elibrary:	29473014
Chemical Abstracts:	2016:1241423
OpenAlex:	W2487467103

DB	Citing
Web of science	14
Scopus	15
Elibrary	13
OpenAlex	17