Sciact
  • EN
  • RU

Mössbauer Study of the Magnetic Transition in ϵ-Fe2O3 Nanoparticles Using Synchrotron and Radionuclide Sources Full article

Journal Journal of Experimental and Theoretical Physics Letters (JETP Letters)
ISSN: 0021-3640 , E-ISSN: 1090-6487
Output data Year: 2019, Volume: 110, Number: 9, Pages: 613-617 Pages count : 5 DOI: 10.1134/S0021364019210082
Tags NUCLEAR RESONANT SCATTERING; HIGH-TEMPERATURE; RAYS
Authors Knyazev Yu.V. 1 , Chumakov A.I. 2 , Dubrovskiy A.A. 1 , Semenov S.V. 1 , Yakushkin S.S. 3 , Kirillov V.L. 3 , Martyanov O.N. 3 , Balaev D.A. 1
Affiliations
1 Kirensky Institute of Physics, Siberian Branch, Russian Academy of Sciences, Krasnoyarsk, 660036 Russia
2 European Synchrotron Radiation Facility (ESRF), F-38043 Grenoble Cedex 9, France
3 Boreskov Institute of Catalysis, Siberian Branch, Russian Academy of Sciences, Novosibirsk, 630090 Russia

Funding (1)

1 Russian Science Foundation 17-12-01111

Abstract: Nuclear γ-resonance experiments with energy and time resolved detection are carried out with ϵ-F2O3 nanoparticles and a 57Co(Rh) laboratory Mössbauer source of γ radiation and a 14.4125 keV synchrotron radiation source on the ID18 beamline (ESRF) in the temperature range of 4–300 K. Both methods show a tremendous increase in the hyperfine field in tetrahedrally coordinated iron positions during the magnetic transition in the range of 80–150 K. As a result, the splitting of the quantum beat peaks in the nuclear scattering spectra is observed in the time interval of 20–170 ns with a periodicity of ∼ 30 ns. In addition, the first quantum beat is slightly shifted to shorter times. A correlation between the quadrupole shift and the orbital angular momentum of iron in ϵ-F2O3 nanoparticles is found. The magnetic transition leads to the rotation of the magnetic moment in the tetrahedral positions of iron around the axis of the electric field gradient by an angle of 44°. © 2019, Pleiades Publishing, Inc.
Cite: Knyazev Y.V. , Chumakov A.I. , Dubrovskiy A.A. , Semenov S.V. , Yakushkin S.S. , Kirillov V.L. , Martyanov O.N. , Balaev D.A.
Mössbauer Study of the Magnetic Transition in ϵ-Fe2O3 Nanoparticles Using Synchrotron and Radionuclide Sources
Journal of Experimental and Theoretical Physics Letters (JETP Letters). 2019. V.110. N9. P.613-617. DOI: 10.1134/S0021364019210082 WOS Scopus РИНЦ AN OpenAlex
Original: Князев Ю.В. , Чумаков А.И. , Дубровский А.А. , Семенов С.В. , Якушкин С.С. , Кириллов В.Л. , Мартьянов О.Н. , Балаев Д.А.
Мессбауэровские исследования магнитного перехода в наночастицах ǫ-Fe2O3 на синхротронном и радионуклидном источниках
Письма в Журнал экспериментальной и теоретической физики. 2019. Т.110. №9. С.614-619. DOI: 10.1134037027419210082 РИНЦ
Dates:
Submitted: Sep 26, 2019
Accepted: Oct 4, 2019
Published print: Nov 1, 2019
Published online: Jan 4, 2020
Identifiers:
Web of science: WOS:000511164800008
Scopus: 2-s2.0-85077637717
Elibrary: 43226246
Chemical Abstracts: 2020:35654
OpenAlex: W2998463902
Citing:
DB Citing
Scopus 5
Web of science 4
Elibrary 8
OpenAlex 5
Altmetrics: