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Factors Affecting Conversion of Methane-Hydrogen Mixtures into Nanostructured Carbon and Hydrogen Научная публикация

Журнал International Journal of Hydrogen Energy
ISSN: 0360-3199 , E-ISSN: 1879-3487
Вых. Данные Год: 2024, Том: 82, Страницы: 662-672 Страниц : 11 DOI: 10.1016/j.ijhydene.2024.07.455
Ключевые слова Catalytic decomposition of methane; Hydrogen production; Carbon nanofibers; Nickel–copper catalyst; Simulation
Авторы Shelepova Ekaterina V. 1 , Maksimova Tatiana A. 1 , Bauman Yury I. 1 , Ayupov Artem B. 1 , Mishakov Ilya V. 1 , Vedyagin Aleksey A. 1
Организации
1 Boreskov Institute of Catalysis, 5 ac. Lavrentieva Ave., 630090, Novosibirsk, Russia

Информация о финансировании (1)

1 Российский научный фонд
Министерство науки и инновационной политики Новосибирской области
24-29-20095

Реферат: At the catalytic decomposition of methane, along with hydrogen, it is possible to obtain carbon nanofibers. The addition of hydrogen to the initial reaction mixture makes it possible to increase significantly the efficiency of the overall process by minimizing the contribution of the catalyst deactivation process caused by coking. As found, the maximum yields of hydrogen and nanostructured carbon over the NiO–CuO/Al2O3 catalyst is achieved at an inlet hydrogen concentration of 13 vol%. The accumulated carbon is represented by well-structured carbon nanofibers, which are resistant to the gasification reaction. The original stacked structure is preserved after the treatment of these fibers in a hydrogen medium. Using numerical methods, the hydrogen productivity at 610 °C was found to be 49.3 mL/(mgcat·h) at an optimal value of the residence time of 5 × 10−3 s.
Библиографическая ссылка: Shelepova E.V. , Maksimova T.A. , Bauman Y.I. , Ayupov A.B. , Mishakov I.V. , Vedyagin A.A.
Factors Affecting Conversion of Methane-Hydrogen Mixtures into Nanostructured Carbon and Hydrogen
International Journal of Hydrogen Energy. 2024. V.82. P.662-672. DOI: 10.1016/j.ijhydene.2024.07.455 WOS Scopus CAPlus OpenAlex
Даты:
Поступила в редакцию: 2 мая 2024 г.
Принята к публикации: 31 июл. 2024 г.
Опубликована online: 3 авг. 2024 г.
Опубликована в печати: 11 сент. 2024 г.
Идентификаторы БД:
Web of science: WOS:001288199100001
Scopus: 2-s2.0-85200162133
Chemical Abstracts: 2024:1702063
OpenAlex: W4401283333
Цитирование в БД:
БД Цитирований
OpenAlex 1
Scopus 2
Web of science 1
Альметрики: