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Mathematical Modelling of a Reverse Flow Reactor with Catalytic Surface Dynamics Full article

Journal Chemical Engineering Science
ISSN: 0009-2509 , E-ISSN: 1873-4405
Output data Year: 2002, Volume: 57, Number: 3, Pages: 393-407 Pages count : 15 DOI: 10.1016/S0009-2509(01)00408-0
Tags Mathematical modelling, Nonlinear dynamics, Reverse flow
Authors Smith Warren R. 1 , Bobrova Ludmilla N. 2
Affiliations
1 School of Mathematics and Statistics, The University of Birmingham, Edgbaston, Birmingham B15 2TT, UK
2 Department of Chemical Engineering, Technische Universiteit Eindhoven, P.O. Box 513, 5600 MB Eindhoven, The Netherlands

Abstract: This paper studies a system of partial differential equations modelling the behaviour of a reverse flow reactor. For the parameters appropriate for the oxidation of ammonia on a Pt/Al2O3 catalyst in a typical laboratory set-up, the reactor may be split into regions where approximate formulas that determine its behaviour are deduced. Numerical calculations are presented and can be used to compare with the analytical formulas. The physical insight gained from the asymptotic analysis suggests a new switching strategy which is the subject of numerical experiments. The switching strategy is found to be efficient at minimising the ammonia exiting the reactor after reversal.
Cite: Smith W.R. , Bobrova L.N.
Mathematical Modelling of a Reverse Flow Reactor with Catalytic Surface Dynamics
Chemical Engineering Science. 2002. V.57. N3. P.393-407. DOI: 10.1016/S0009-2509(01)00408-0 WOS Scopus РИНЦ OpenAlex ANCAN
Dates:
Submitted: Feb 4, 2000
Accepted: Aug 21, 2001
Published online: Dec 7, 2001
Published print: Feb 1, 2002
Identifiers:
≡ Web of science: WOS:000173714900009
≡ Scopus: 2-s2.0-0037169346
≡ Elibrary: 13952054
≡ OpenAlex: W2015234882
≡ Chemical Abstracts: 2002:64844
≡ Chemical Abstracts (print): 136:202493
Citing:
≡ Web of science 6 Сбор данных от 13.02.2026
≡ Scopus 8 Сбор данных от 08.02.2026
≡ OpenAlex 6 Сбор данных от 08.02.2026
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