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Simulation of Diesel Autothermal Reforming over Rh/Ce0.75Zr0.25O2-δ-η-Al2O3/FeCrAl Wire Mesh Honeycomb Catalytic Module Научная публикация

Общее Язык: Английский, Жанр: Статья (Full article),
Статус опубликования: Опубликована, Оригинальность: Оригинальная
Журнал Chemical Engineering and Processing: Process Intensification
ISSN: 0255-2701
Вых. Данные Год: 2020, Том: 150, Номер статьи : 107876, Страниц : 7 DOI: 10.1016/j.cep.2020.107876
Ключевые слова Autothermal reforming; Diesel; rhodium; Zirconia-ceria; Structured catalyst; wire metal mesh
Авторы Zazhigalov S.V. 1 , Rogozhnikov V.N. 1 , Snytnikov P.V. 1 , Potemkin D.I. 1 , Simonov P.A. 1 , Shilov V.A. 1,2 , Ruban N.V. 1,2 , Kulikov A.V. 1 , Zagoruiko A.N. 1 , Sobyanin V.A. 1
Организации
1 Boreskov Institute of Catalysis, Pr. Akademika Lavrentieva, 5, Novosibirsk, 630090, Russia
2 Novosibirsk State University, PirogovaSt., 2, Novosibirsk, 630090, Russia

Информация о финансировании (1)

1 Российский научный фонд 19-19-00257

Реферат: The study was dedicated to the mathematical modeling of the catalytic autothermal reforming (ATR) of diesel fuel – effective method for hydrogen production. The structured wire mesh Rh/Ce0.75Zr0.25O2-δ-η-Al2O3/FeCrAl catalyst was tested in pilot scale reactor and showed high efficiency in studied diesel autothermal reaction conditions. The process simulation was carried out by commercial software COMSOL Multiphysics in 2D axisymmetric geometry. The catalyst module was simulated as homogeneous porous medium. Reaction model included diesel oxidation, diesel steam reforming, water-gas shift reaction, CO methanation, CO oxidation and hydrogen oxidation. Fitting the experimental results including product distribution and temperature profile allowed to define the kinetic parameters corresponding to the best fit. The suggested simple quasi-homogeneous model describes experimental results (module temperature and outlet gas composition) with a good accuracy and could be used for process optimization and up-scaling.
Библиографическая ссылка: Zazhigalov S.V. , Rogozhnikov V.N. , Snytnikov P.V. , Potemkin D.I. , Simonov P.A. , Shilov V.A. , Ruban N.V. , Kulikov A.V. , Zagoruiko A.N. , Sobyanin V.A.
Simulation of Diesel Autothermal Reforming over Rh/Ce0.75Zr0.25O2-δ-η-Al2O3/FeCrAl Wire Mesh Honeycomb Catalytic Module
Chemical Engineering and Processing: Process Intensification. 2020. V.150. 107876 :1-7. DOI: 10.1016/j.cep.2020.107876 WOS Scopus РИНЦ
Даты:
Поступила в редакцию: 9 сент. 2019 г.
Принята к публикации: 26 февр. 2020 г.
Опубликована online: 27 февр. 2020 г.
Опубликована в печати: 1 апр. 2020 г.
Идентификаторы:
Web of science WOS:000547817900009
Scopus 2-s2.0-85080992160
РИНЦ 43247330
Chemical Abstracts 2020:455904
Альметрики: